Physics and Astronomy Faculty Publications

Document Type

Article

Abstract

A general strategy for low-temperature processing of colloidal nanocrystals into all-inorganic films is reported. The present methodology goes beyond the traditional ligand-interlinking scheme and relies on encapsulation of morphologically defined nanocrystal arrays into a matrix of a wide-band gap semiconductor, which preserves optoelectronic properties of individual nanoparticles while rendering the nanocrystal film photoconductive. Fabricated solids exhibit excellent thermal stability, which is attributed to the heteroepitaxial structure of nanocrystal matrix interfaces, and show compelling light-harvesting performance in prototype solar cells.

Publication Date

12-2011

Publication Title

Journal Of The American Chemical Society

Volume

133

Issue

50

Start Page No.

20488

End Page No.

20499

DOI

10.1021/ja208670r

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